Strong field single ionization of homo- and heteronuclear noble gas dimers with ultrashort infrared laser pulses is experimentally investigated. A pronounced photoelectron yield maximum is found for dimers in the momentum range |p|≤0.1  a.u. which is absent for the corresponding monomer. This yield enhancement can be attributed to a new two-step strong field ionization mechanism active only in the dimers. In the first step, frustrated tunnel ionization at one of the atomic centers populates Rydberg states, which then become ionized in a second step through charge oscillation within the dimer ion core.

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