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Reduced graphene
oxide (rGO) is an ideal candidate for the improvement
of supercapacitor (SC) performances due to its industrial-ready manufacturing
process and ease of processing. In this work, rGO was used as an active
binder for the manufacture of carbon black (CB) and rGO-based SCs.
Being able to form a stable suspension in water, graphene oxide (GO)
was initially exploited as a dispersing agent to fabricate a homogeneous
slurry with CB having exclusively water as a low-cost and environment-friendly
solvent. After casting on a suitable substrate, the material was subjected
to thermal treatment allowing the reduction of GO to rGO, which was
successively confirmed by chemical–physical analysis. An innovative
current collector, consisting of high-quality rGO paper, was also
proposed ensuring an improved adhesion between the active material
and the substrate and a reduction of the whole weight with respect
to devices fabricated using common metallic current collectors. Due
to the interesting electrochemical performances, with a high specific
power of 32.1 kW kg
–1
and a corresponding specific
energy of 8.8 Wh kg
–1
at a current of 1 A g
–1
, and the improved manufacturing process, the described
“all-graphene-based” device represents a valuable candidate
for the future of SCs.
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