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Rapid Access to Reactive Methanimines by the Retro-Ene Reaction: The Photoelectron Spectrum of N-Dimethylsilylmethanimine. -An improved synthesis of the parent compound (II), trapped as thioether (IV), and similarly of silyl derivative (VII) is achieved by flash vacuum thermolysis of amines (I) or (V). -(SYSTERMANS, A.; LEFEVRE, V.; RIPOLL, J.-L.; PIEPLU, T.; HOGGAN, P. E.; JOANTEGUY, S.; CHROSTOWSKA-SENIO, A.; PFISTER-GUILLOUZO, G.; New J. Chem. 21 (1997) 3, 383-387; Lab. Chim. Mol. Thio-Org., CNRS, Inst. Sci. Matiere Rayonnem., Univ. Caen, F-14050 Caen, Fr.; EN)