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This study investigates the interference alignment techniques for cognitive radio networks toward 5G to meet the demand and challenges for future wireless communications requirements. In this context, we examine the performance of the interference alignment in two parts. In the first part of this chapter, a multi-input multi-output (MIMO) cognitive radio network in the presence of multiple secondary users (SUs) is investigated. The proposed model assumes that linear interference alignment is used at the primary system to lessen the interference between primary and secondary networks. Herein, we derive the closed-form mathematical equations for the outage probability considering the interference leakage occurred in the primary system. The second part of this study analyzes the performance of interference alignment for underlay cognitive two-way relay networks with channel state information (CSI) quantization error. Here, a two-way amplify-and-forward relaying scheme is considered for independent and identically distributed Rayleigh fading channel. The closed-form average pairwise error probability expressions are derived, and the effect of CSI quantization error is analyzed based on the bit error rate performance. Finally, we evaluate the instantaneous capacity for both primary and secondary networks * .