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In a head-to-head study, ILs based upon tetraarylphosphonium cations exhibit superior long-term thermal stability compared to familiar salts based upon imidazolium, quaternary ammonium, or tetraalkylphosphonium cations.

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The synthesis of a series of new lipid-inspired ionic liquids through thiol-ene "click" reaction with a single-step process. This synthesis offers considerable promise as an efficient and orthogonal method to construct structurally diverse imidazolium-type ionic liquids with linear and branched cationic tails, as well as versatility in the placement of the sulfur heteroatom. Profound solvent effect in this ene reaction regioselectivity has been observed.