Structural optimizations of the piezoelectric layer in nanogenerators have been predicted to enhance the output performance in terms of the figure of merit. Here, we report the effect of dielectric constant on electrical outputs of piezoelectric nanogenerator using ZnO/PDMS composites with varied ZnO coverages. The dielectric constant of piezoelectric layers was adjusted from 3.37 to 6.75. The electrical output voltage of 9 mV was achieved in the nanogenerator containing the ZnO/PDMS composite with the dielectric constant of 3.46, which is an 11.3-fold enhancement compared to the value of the nanogenerator featuring the composite with high dielectric constants. Significantly, lowering the dielectric constant of the piezoelectric layer improves the electrical output performance of piezoelectric nanogenerators.

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