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Plasma technology is considered a sustainable and clean technology for the conversion of naturally abundant compounds (i.e., water (H2O) and nitrogen gas (N2)) into energy-abundant compounds (e.g., hydrogen gas (H2), ammonia (NH3)) or chemical feed molecules (e.g., nitric oxide (NO)). Here, we report a plasma catalyst-integrated system for sustainable ammonia production, which can facilitate massive, localized ammonia production. This study demonstrates the single-step cogeneration of H2 and nitric oxides (NO x ) from H2O in the nitrogen discharge used for ammonia production, which proceeded via the catalytic reduction of NO x by H2. The proposed plasma technique yields higher NO and H2 concentrations than conventional plasma methods, which were used to obtain an ammonia concentration of ∼0.84% with a selectivity of ∼95% and a production rate of 120 μmol/s. These promising results provide a breakthrough in the transition toward sustainable and environmentally friendly ammonia production.