The widely available and easily accessible natural resources are very important to remove organic dyes from wastewater. Here in this work, Methyele Blue (MB) removal efficiency of Jemma Silica Sand (JSS) and Sugar Cane Bagasse ash (SCBA) from aqueous solutions was investigated. The XRD patterns revealed that both JSS and SCBA are crystalline, but the crystalline size of JSS is 56.27 nm and that of SCBA is 70.90 nm. In addition to the percentage of silicon dioxide in JSS was 98% and in that of SCBA was 71.5% as confirmed by XRF results. The morphology and elemental composition of the two materials were revealed by SEM and EDX. The MB removal efficiency of SCBA (~99.14%) is greater than that of JSS (~93.75) because of its higher porosities nature. The adsorption of MB by SCBA follows the Freundlich isotherm model and pseudo-second-order kinetic model indicating chemisorption. Therefore, SCBA is promising absorbent for removing MB from wastewater because of its efficient, cost-effectiveness, and environmentally friendly nature.