Davidson, N.C.; presently a visiting member of the ORNL Chemistry Division. NOTICE This document contains information of a preliminary nature. It if wbjaet to reVsion or correction and therefore does not represent a fine' report. The project was administered by the Office of Nuclear Waste Isolation, Battelle Memorial Institute. OAK RIDGE NATIONAL LABORATORY Oak Ridge, Tennessee 37830 operated by UNION CARBIDE CORPORATION for the DEPARTMENT OF ENERGY nonet Tn» rtprHi WM praired * *n accow of work •pmiM»vdhyl>ttUittft4&lkiC.tfi«*iiflmi NfKrKrrAf Univi S«« nor dw Uoitrt 5r*e* OtyTmi of ti*\0. nor jny of Act fmploTW*. m* my of tmt comracfors. Bbcontticfcm. or r*cw flnptotvM. "fc** •*> wwrMtly. npvcm or mpM. of am-toWtty or rapoMbditr for *t *car«icy. or wfvfef* of My mfomtmn. mpmwm. proit prom d«ckMtd. or repranti fctt itt wx «TMM •nrVfr prlMHly owwd neitt.
and mineralogy of the Vacherie and Raybum salt doses ' 13 2.2.2 Fluid Inclusions in the salt 14 3. THEORETICAL ASPECTS OF LIOOID BRINE MIGRATION WITHIN CRYSTALS OF HaCl 15 3.1 Brine Migration Induced by a Thermal Gradient 15 3.1.1 Introduction. 15 3.1.2 Anthony and Cline equation for brine migration velocity 16 3.1.3 Rearrangement of Anthony and Cline equation to include the empirical relationship between migration velocity ,and kinetic potential .... 18 3.1.4 Theoretical equations of Geguzin and later workers 3.1.5 Thermodynamic relationship between kinetic potential and interface concentration 3.1.6 Derivation of the transport equation with thermal diffusion and applications 3.1.7 Theoretical equations assuming nonlinear interface kinetics 24 3.1.8 Numerical values of the migration equation parameters 3.1.9 Predicted maximum ratei of migration, Vxnax> of brine inclusions in single crystals of NaCl ... 3.1.10 Ratio (V/V,^) of calculated migration velocity to maximum migration velocity: effects of kinetic potential ...... j4 3.1.11 Effects of kinetic potential 3.2 Effects of Stress and of Gamma Irradiation on Kinetic Potential 4. MIGRATION RATE DATA FOR LIQUID BRINE INCLUSIONS IN SINGLE CRYSTALS OF NaCl 4.1 Natural Crystals of Bedded Salt with Natural Brine Inclusions 4.1.1 Data for bedded salt in the Carey mine, Hutchinson, Kansas 4.1.2 Data for bedded salt in SENM (ERDA Core 9) ... 4.1.3 Data for bedded salt in the Carey mine at Lyons, Kansas ............. 4.1.4 Data for bedded salt In SENM (near Salt Block II site) 4.1.5 Effects of stored radiation energy on brine migration .................... 4.1.6 Evidence that the kinetic potential has a finite value at zero migration rate ....... V 4.2 Natural Crystals of Dome Salt with Natural Brine Inclusions 48 4.3 Synthetic NaCI with Inclusions of Pure NaCI Brine ... 48 4.4 Summary of Information on Maximum Rates of Migration of Brine Inclusions in Bedded Salt 49 4.4.1 Kinetic potential effects 49 4.4.2 Shape of brine inclusions 50 4.4.3 Other effects of gamma radiation ..
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