Perpendicular exchange bias was investigated using Pt/Co/α-Cr2O3(0001) thin films prepared by a reactive DC magnetron sputtering method. On the α-Cr2O3(0001) layer, the Pt/Co thin film simultaneously showed perpendicular magnetic anisotropy (PMA) and perpendicular exchange bias (PEB). Although PEB was not observed at room temperature, it suddenly appeared, accompanied by a unique temperature dependence. The suddenly appearing PEB was as large as a unidirectional magnetic anisotropy energy, JK, of about 0.29 erg/cm2. The mechanism of the sudden appearance of JK is discussed on the basis of Meiklejohn and Bean's exchange anisotropy model.

By using the perpendicular-exchange-biased Pt/Co/α-Cr(2)O(3) system, we provide experimental evidence that the unreversed uncompensated Cr spins exist at the Co/α-Cr(2)O(3) interface. The unreversed uncompensated Cr spin manifests itself in both the vertical shift of an element-specific magnetization curve and the relative peak intensity of soft-x-ray magnetic circular dichroism spectrum. We also demonstrate an in situ switching of the interfacial Cr spins and correspondingly a reversal of the exchange bias without interfacial atomic diffusion. Such switching shows the direct relationship between the interfacial antiferromagnetic spins and origin of the exchange bias. The demonstrated switching of exchange bias would likely offer a new design of advanced spintronics devices, using the perpendicular-exchange-biased system, with low power consumption and ultrafast operation.

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We investigated perpendicular magnetic anisotropy and exchange magnetic anisotropy in a Pt/Co/ a-Cr 2 O 3 (0001) thin film grown on an a-Al 2 O 3 (0001) substrate. The film exhibits perpendicular magnetic anisotropy below a Co thickness of 1.2 nm at room temperature. Independent of the magnetic easy direction of the Co layer, the perpendicular exchange bias (PEB) appears in a direction perpendicular to the film below 80 K. The maximum unidirectional magnetic anisotropy energy estimated from the exchange bias field is 0.33 erg/cm 2 , which is higher than the reported PEB strength. The perpendicular exchange bias is accompanied by the in-plane remanent magnetization and an increase in the in-plane coercivity. We speculate that the increases in the in-plane remanent magnetization and the in-plane coercivity are caused by the spin canting of Cr 3þ in the a-Cr 2 O 3 (0001) layer. V