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Image-based closed-loop tracking (IBCLT) is an important part of the process of target tracking. The Risley prism system has a unique advantage in improving the target tracking ability because of its compact and lightweight structure. Compared with traditional target tracking equipment, the Risley prism system has two difficulties in the process of IBCLT. First, the Risley prism is a complex coupling system of double input and double output. Second, the Risley prism itself is a nonlinear system. These problems lead to decrease in dynamic response and inconsistent target tracking capabilities. Thus, this paper proposes a method to implement multivariable decoupling and reduce the nonlinear effect. First, the boresight error of IBCLT is decoupled to the azimuth and elevation directions by the rotation matrix error-decoupling (RMED) method. Second, the gains of IBCLT in azimuth and elevation directions are independent variables that comes from two functions of the target elevation angle. The experimental results show that the IBCLT error deviation of different static targets in the field of view is within 0.025 arcsec, which is 70% lower compared with the fixed gain method. Furthermore, the steady-state error deviation of moving targets is controlled within 2.5 arcsec. These experimental results prove the feasibility and effectiveness of the proposed method.