In recent years, there has been dramatic progress in the photonics field in disordered media, ranging from applications in solar collectors, photocatalyzers, random lasing, and other novel photonic functions, to investigations into fundamental topics, such as light confinement and other phenomena involving photon interactions. This paper reports several pieces of experimental evidence of localization transition in a strongly disordered scattering medium composed of a colloidal suspension of core-shell nanoparticles (TiO2@silica) in ethanol solution. We demonstrate the crossover from a diffusive transport to a localization transition regime as the nanoparticle concentration is increased, and that an enhanced absorption effect arises at localization transition.
Anderson localization
of light and random lasing in this critical
regime is an open research frontier, which besides being a basic research
topic could also lead to important applications. This article investigates
the random laser action at the localization transition in a strongly
disordered scattering medium composed of a colloidal suspension of
core–shell nanoparticles (TiO
2
@Silica) in ethanol
solution of Rhodamine 6G. The classical superfluorescence band of
the random laser was measured separately by collecting the emission
at the back of the samples, showing a linear dependence with pumping
fluence without gain depletion. However, frontal collection showed
saturation of the absorption and emission. Narrow peaks of approximately
equal intensity are observed on top of the classical superfluorescence
band, indicating suppression of the interaction between the peaks
modes. The linewidth of these peaks is lower than that of the passive
modes of the scattering medium. A method called fraction of absorbed
pumping allowed us to infer that this peak’s mode (localized
modes) is confined to a shallow region near the input-pumping border.
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