The advanced molybdenum-based rare process experiment (AMoRE) aims to search for neutrinoless double beta decay ($$0\nu \beta \beta $$0νββ) of $$^{100}$$100Mo with $$\sim 100\,\hbox {kg}$$∼100kg of $$^{100}$$100Mo-enriched molybdenum embedded in cryogenic detectors with a dual heat and light readout. At the current, pilot stage of the AMoRE project we employ six calcium molybdate crystals with a total mass of 1.9 kg, produced from $$^{48}$$48Ca-depleted calcium and $$^{100}$$100Mo-enriched molybdenum ($$^{48{{\text {depl}}}}\hbox {Ca}^{100}\hbox {MoO}_{4}$$48deplCa100MoO4). The simultaneous detection of heat (phonon) and scintillation (photon) signals is realized with high resolution metallic magnetic calorimeter sensors that operate at milli-Kelvin temperatures. This stage of the project is carried out in the Yangyang underground laboratory at a depth of 700 m. We report first results from the AMoRE-Pilot $$0\nu \beta \beta $$0νββ search with a 111 kg day live exposure of $$^{48{{\text {depl}}}}\hbox {Ca}^{100}\hbox {MoO}_{4}$$48deplCa100MoO4 crystals. No evidence for $$0\nu \beta \beta $$0νββ decay of $$^{100}$$100Mo is found, and a upper limit is set for the half-life of $$0\nu \beta \beta $$0νββ of $$^{100}$$100Mo of $$T^{0\nu }_{1/2} > 9.5\times 10^{22}~\hbox {years}$$T1/20ν>9.5×1022years at 90% C.L. This limit corresponds to an effective Majorana neutrino mass limit in the range $$\langle m_{\beta \beta }\rangle \le (1.2-2.1)\,\hbox {eV}$$⟨mββ⟩≤(1.2-2.1)eV.

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