Die Strukturbestimmung an Einkristallen ergibt für Ba2S3 eine tetragonale Symmetrie mit I41md, a = 6,112, c = 15,950 Å, Z=4 und für BaS3 ebenfalls eine tetragonale Struktur mit P421m, a = 6,871, c =4,168 A und z = 2. Ba2S3 enthält ein Sulfidion und ein S2(2‐)‐Polysulfidion.
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