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The novel and sensitive In-Gas Laser Ionization Spectroscopy (IGLIS) technique enables high-precision laser spectroscopy of the heaviest elements and isotopes very far from stability that are produced in fusion-evaporation reactions at in-flight separators. Powerful and dedicated laser systems are required in these facilities to realize in-gas jet laser spectroscopy with optimal spectral resolution and efficiency. The performance with respect to the requirements for IGLIS studies at the low energy front-end of the Super Separator Spectrometer (S 3 ) at GANIL, France, of Dye and Ti:sapphire laser systems is investigated. In addition, a number of specific experimental cases on key isotopes of the elements Ag, Sn, Ac, and No are discussed in detail.

Hot cavity resonant ionization laser ion sources (RILIS) provide a multitude of radioactive ion beams with high ionization efficiency and element selective ionization. However, in hot cavity RILIS there still remains isobaric contaminations in the extracted beam from surface ionized species. An ion guide-laser ion source (IG-LIS) has been implemented that decouples the hot isotope production region from the laser ionization volume. A number of IG-LIS runs have been conducted to provide isobar free radioactive ion beams for experiments. Isobar suppression of up to 10 6 has been achieved, however, IG-LIS still suffers from an intensity loss of 50-100 × as compared to hot cavity RILIS. Operating parameters for IG-LIS are being optimized and design improvements are being implemented into the prototype for robust and efficient on-line operation. Recent SIMION ion optics simulation results and the ongoing development status of the IG-LIS are presented.

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We present the first results obtained from the S3 Low-Energy Branch , the gas cell setup at SPIRAL2-GANIL, which will be installed behind the S3 spectrometer for atomic and nuclear spectroscopy studies of exotic nuclei. The installation is currently being commissioned offline, with the aim to establish optimum conditions for the operation of the radio frequency quadrupole ion guides, mass separation and ion bunching, providing high-efficiency and low-energy spatial spread for the isotopes of interest. Transmission and mass-resolving power measurements are presented for the different components of the S3-LEB setup. In addition, a single-longitudinal-mode, injection-locked, pumped pulsed-titanium–sapphire laser system has been recently implemented and is used for the first proof-of-principle measurements in an offline laser laboratory. Laser spectroscopy measurements of erbium, which is the commissioning case of the S3 spectrometer, are presented using the 4f126s23H6→4f12(3H)6s6p optical transition.