Two-dimensional (2D) materials for their versatile band structures and strictly 2D nature have attracted considerable attention over the past decade. Graphene is a robust material for spintronics owing to its weak spin-orbit and hyperfine interactions, while monolayer transition metal dichalcogenides (TMDs) possess a Zeeman effect-like band splitting in which the spin and valley degrees of freedom are nondegenerate. The surface states of topological insulators (TIs) exhibit a spinmomentum locking that opens up the possibility of controlling the spin degree of freedom in the absence of an external magnetic field. Nanostructures made of these materials are also viable for use in quantum computing applications involving the superposition and entanglement of individual charge and spin quanta. In this article, we review a selection of transport studies addressing the confinement and manipulation of charges in nanostructures fabricated from various 2D materials. We supply the entry-level knowledge for this field by first introducing the fundamental properties of 2D bulk materials followed by the theoretical background relevant to the physics of nanostructures. Subsequently, a historical review of experimental development in this field is presented, from the early demonstration of graphene nanodevices on SiO2 substrate to more recent progress in utilizing hexagonal boron nitride to reduce substrate disorder. In the second part of this article, we extend our discussion to TMDs and TI nanostructures. We aim to outline the current challenges and suggest how future work will be geared towards developing spin qubits in 2D materials.
Weyl semimetals have drawn considerable attention for their exotic topological properties in many research fields. When in combination with s-wave superconductors, the supercurrent can be carried by their topological surface channels, forming junctions mimicking the behavior of Majorana bound states. Here, we present a transmon-like superconducting quantum intereference device (SQUID) consisting of lateral junctions made of Weyl semimetal Td−MoTe 2 and superconducting leads of niobium nitride (NbN). The SQUID is coupled to a readout cavity made of molybdenum rhenium (MoRe), whose response at high power reveals the existence of the constituting Josephson junctions (JJs). The loop geometry of the circuit allows the resonant frequency of the readout cavity to be tuned by the magnetic flux. We demonstrate a JJ made of MoTe 2 and a flux-tunable transmonlike circuit based on Weyl semimetals. Our study provides a platform to utilize topological materials in SQUID-based quantum circuits for potential applications in quantum information processing.
We performed a series of theoretical transport studies on Y-branch electron waveguides which are embedded in mid-size armchair graphene nanoribbons. Non-equilibrium Green's function with different approximations of tight-binding Hamiltonian has been employed. Using the first nearest hopping approximation, we observed very pronounced conductance quantization, the structure of which depends on geometrical design and shows a spacing of 4e /h, indicating the existence of valley degree of freedom. Moreover, by incorporating the third nearest approximation, we observed seminal plateaus deviated from multiples of 4e/h conductance, suggesting the lift of valley degeneracy. Finally, Quasi-one dimensional band structure calculations have been performed to study the availability of energy channels and the role of the major geometrical parameters on the transport.
Monolayer transition-metal dichalcogenides (TMDs) are considered to be fantastic building blocks for a wide variety of optical and optoelectronic devices such as sensors, photodetectors, and quantum emitters, owing to their direct band gap, transparency, and mechanical flexibility. The core element of many conventional electronic and optoelectronic devices is the p-n junction, in which the p-and n-types of the semiconductor are formed by chemical doping in different regions.Here, we report a series of optoelectronic studies on a monolayer WSe 2 in-plane p-n photodetector, demonstrating a lowpower dissipation by showing an ambipolar behavior with a reduced threshold voltage by a factor of two compared with the previous results on a lateral electrostatically doped WSe 2 p-n junction. The fabrication of the device is based on a polycarbonates (PC) transfer technique and hence no electron-beam exposure induced damage to the monolayer WSe 2 is expected. Upon optical excitation, the photodetector demonstrates a photoresponsivity of 0.12 mA•W −1 and a maximum external quantum efficiency of 0.03%. Our study provides an alternative platform for a flexible and transparent twodimensional photodetector, from which we expect to further promote the development of next-generation optoelectronic devices.
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