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A natural dispersant exhibiting recyclable buffer property is obtained from aqueous extract of Balanites roxburghii fruit and used as a highly efficient catalytic medium for C–C bond construction via Knoevenagel condensation and tandem Knoevenagel–Michael reaction.

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A library of quinazolinones was prepared by the one-pot three-component reaction of isatoic anhydride, ammonium salts/amines, and various electrophiles using aqueous hydrotropic solution as an efficient, economical, reusable, and green medium giving good to excellent yields of products in very short time. The method offers a versatile way for the development of diversity-oriented synthesis of quinazolinones.