No abstract

No abstract

No abstract

Abstract. Temporal variations in the amount of radionuclides released into the atmosphere during the Fukushima Daiichi Nuclear Power Station (FNPS1) accident and their atmospheric and marine dispersion are essential to evaluate the environmental impacts and resultant radiological doses to the public. In this paper, we estimate the detailed atmospheric releases during the accident using a reverse estimation method which calculates the release rates of radionuclides by comparing measurements of air concentration of a radionuclide or its dose rate in the environment with the ones calculated by atmospheric and oceanic transport, dispersion and deposition models. The atmospheric and oceanic models used are WSPEEDI-II (Worldwide version of System for Prediction of Environmental Emergency Dose Information) and SEA-GEARN-FDM (Finite difference oceanic dispersion model), both developed by the authors. A sophisticated deposition scheme, which deals with dry and fog-water depositions, cloud condensation nuclei (CCN) activation, and subsequent wet scavenging due to mixed-phase cloud microphysics (in-cloud scavenging) for radioactive iodine gas (I2 and CH3I) and other particles (CsI, Cs, and Te), was incorporated into WSPEEDI-II to improve the surface deposition calculations. The results revealed that the major releases of radionuclides due to the FNPS1 accident occurred in the following periods during March 2011: the afternoon of 12 March due to the wet venting and hydrogen explosion at Unit 1, midnight of 14 March when the SRV (safety relief valve) was opened three times at Unit 2, the morning and night of 15 March, and the morning of 16 March. According to the simulation results, the highest radioactive contamination areas around FNPS1 were created from 15 to 16 March by complicated interactions among rainfall, plume movements, and the temporal variation of release rates. The simulation by WSPEEDI-II using the new source term reproduced the local and regional patterns of cumulative surface deposition of total 131I and 137Cs and air dose rate obtained by airborne surveys. The new source term was also tested using three atmospheric dispersion models (Modèle Lagrangien de Dispersion de Particules d'ordre zéro: MLDP0, Hybrid Single Particle Lagrangian Integrated Trajectory Model: HYSPLIT, and Met Office's Numerical Atmospheric-dispersion Modelling Environment: NAME) for regional and global calculations, and the calculated results showed good agreement with observed air concentration and surface deposition of 137Cs in eastern Japan.

The source term of the atmospheric release of 131 I and 137 Cs due to the Fukushima Dai-ichi Nuclear Power Plant accident estimated by previous studies was validated and refined by coupling atmospheric and oceanic dispersion simulations with observed 134 Cs in seawater collected from the Pacific Ocean. By assuming the same release rate for 134 Cs and 137 Cs, the sea surface concentration of 134 Cs was calculated using the previously estimated source term and was compared with measurement data. The release rate of 137 Cs was refined to reduce underestimation of measurements, which resulted in a larger value than that previously estimated. In addition, the release rate of 131 I was refined to follow the radioactivity ratio of 137 Cs. As a result, the total amounts of 131 I and 137 Cs discharged into the atmosphere from 5 JST on March 12 to 0 JST on March 20 were estimated to be approximately 2.0 × 10 17 and 1.3 × 10 16 Bq, respectively.