As mental health issues increase worldwide, nature-based experiences are being recognized as alternative treatments for improving health and well-being. Increasing urbanization precludes many people from accessing green spaces owing to time or physical limitations. Therefore, opportunities to connect with nature through virtual technology is being encouraged. We conducted a systematic review of studies on the psychological effects of experiencing nature using virtual technology. We searched the academic databases PubMed, Web of Science, and Scopus for relevant studies and assessed their quality using Cochrane’s RoB 2 and ROBINS-I tools. Twenty-one studies were included and the psychological outcomes were negatively synthesized by the intervention characteristics (duration, observation position of the landscape, interaction, environment description, and sensory type). Psychological outcomes were classified into emotional recovery, cognitive recovery, stress reduction, and other indicators. Emotional recovery was most consistently presented, and virtual natural contact alleviated negative emotions more than it elicited positive emotions. Additionally, virtual nature interventions lasting more than 10 min showed more consistent effects than those of less than 10 min. Moreover, an open field of view led to significant emotional recovery and an in-forest view led to significant cognitive recovery. Despite some limitations, our findings will contribute to the development of virtual forest experiences to improve human well-being.