Solar‐driven interfacial steam generation has emerged as an innovative technique for seawater desalination due to its high photothermal conversion efficiency and potential industrial applications. Herein, a superior interfacial heat accumulation structure composed of semiconductive in situ polymerization (polypyrrole) of nickel foam (IPNF) is reported. The IPNF photothermal layer is assembled with superhydrophilic polyurethane substrate for synchronous water transport and excellent thermal insulation. The 2D ultrablack mesh induces multiple incident rays within the diffused polymerized surface, which allows omnidirectional solar absorption (88.5 %) and intensifying heat localization (49.5 °C @ 1 sun). The state‐of‐the‐art evaporation performances reveal that the integrated IPNF solar evaporator exhibits an excellent evaporation rate (1.74 kg m−2 h−1) and solar‐to‐vapor conversion efficiency (90% excluding heat losses) under 1 kW m−2 solar intensity. Besides this, the long‐term evaporation experiments show negligible discrepancy under seawater conditions (13.27 kg m−2/8 h under 1 kW m−2) and engrain its functioning potential for multimedia and salt rejection (3.2 g × NaCl/240 min). More importantly, herein, insights into different water states in the polymeric network systems during solar‐driven evaporation are provided. This work shows a significant potential to generate freshwater excluding heavy metals and other oil emulsions for industrial applications.

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Low-cost and washable resistive switching (RS) memory devices with stable retention and low operational voltage are important for resistive random-access memory (RRAM).

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