We have experimentally demonstrated that because of intensity clamping, when the laser peak power is higher than the critical power for self-focusing, further increase of the laser power cannot result in corresponding increase of the laser ablation rate of a metallic sample placed in gases. The ablation rate will finally approach a stabilized value. Also, the experimental technique implemented in our work could be potentially used to measure the self-focusing critical power and the nonlinear refractive index.

Polycyclic aromatic hydrocarbons (PAHs) are among the most toxic air pollutants in China. However, because there are unsubstantial data on indoor and outdoor particulate PAHs, efforts in assessing inhalation exposure and cancer risk to PAHs are limited in China. This study measured 12 individual PAHs in indoor and outdoor environments at 36 homes during the non-heating period and heating period in 2009. Indoor PAH concentrations were comparable with outdoor environments in the non-heating period, but were lower in the heating period. The average indoor/outdoor ratios in both sampling periods were lower than 1, while the ratios in the non-heating period were higher than those in the heating period. Correlation analysis and coefficient of divergence also verified the difference between indoor and outdoor PAHs, which could be caused by high ventilation in the non-heating period. To support this conclusion, linear and robust regressions were used to estimate the infiltration factor to compare outdoor PAHs to indoor PAHs. The calculated infiltration factors obtained by the two models were similar in the non-heating period but varied greatly in the heating period, which may have been caused by the influence of ventilation. Potential sources were distinguished using a diagnostic ratio and a mixture of coal combustion and traffic emission, which are major sources of PAHs. Practical ImplicationsParticulate PAHs distribution characterizations between indoor and outdoor atmosphere should be implemented in some typical cities, communities or houses. This study will fill the gap of characterizations, relationship and potential sources of outdoor and indoor particulate matter bound PAHs in China, which was rarely reported in previous studies. This study is the first attempt to use the methods of linear and robust regression to estimate the infiltration factors of PAHs. Similar methods were applied only on PM in previous studies. The study also testifies the relationship between ventilation and PAHs indoor-outdoor distribution in several statistical methods.

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