Dioxomolybdenum(vi) complexes including Mo02(dipic)(HMPA) 2a and Mo02(dedtc)* 2b (dipic = 2,6-pyridinedicarboxylate; HMPA = hexamethylphosphoramide; dedtc = N,N-diethyl dithiocarbamate) catalyse the allylic amination of alkenes by phenyl hydroxylamine; the reactions are characterized by a high degree of regioselectivity resulting from double bond migration.
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