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NRC Publications Archive Archives des publications du CNRCThis publication could be one of several versions: author's original, accepted manuscript or the publisher's version. / La version de cette publication peut être l'une des suivantes : la version prépublication de l'auteur, la version acceptée du manuscrit ou la version de l'éditeur. For the publisher's version, please access the DOI link below./ Pour consulter la version de l'éditeur, utilisez le lien DOI ci-dessous.http://doi.org/10.1103/PhysRevLett.100.233603Access and use of this website and the material on it are subject to the Terms and Conditions set forth at Strong field multiphoton inversion of a three-level system using shaped ultrafast laser pulses Clow, Stephen D.; Trallero-Herrero, Carlos; Bergeman, Thomas; Weinacht, Thomas http://nparc.cisti-icist.nrc-cnrc.gc.ca/fra/droits L'accès à ce site Web et l'utilisation de son contenu sont assujettis aux conditions présentées dans le site LISEZ CES CONDITIONS ATTENTIVEMENT AVANT D'UTILISER CE SITE WEB.
NRC Publications Record / Notice d'Archives des publications de CNRC:http://nparc.cisti-icist.nrc-cnrc.gc.ca/eng/view/object/?id=20434406-7191-4bb9-b11b-11b54510b510 http://nparc.cisti-icist.nrc-cnrc.gc.ca/fra/voir/objet/?id=20434406-7191-4bb9-b11b-11b54510b510 We demonstrate strong-field population inversion in a three-level system with single and multiphoton coupling between levels using a single shaped ultrafast laser pulse. Our interpretation of the pulse shape dependence illustrates the difference between sequential population transfer and adiabatic rapid passage in three-level systems with multiphoton coupling between levels.
Strong Field Multiphoton Inversion of a Three-Level System Using Shaped Ultrafast Laser Pulses
We demonstrate a population inversion in a three-level system via three-photon absorption from a single shaped ultrafast laser pulse. The optimal pulse shape for the inversion is discovered using closed-loop learning control and interpreted via pulse shape parameter scans and numerical integration of the Schrödinger equation. The population inversion is measured using a combination of spontaneous and stimulated emissions. Our results illustrate the importance of dynamic Stark shifts in coherent multi-photon excitation.
Wannier functions for a 1D quantum system with a generic periodic potential are calculated directly using orthogonal compact support multiwavelets in conjunction with a sparse iterative method. This allows systematic elimination of error from scales both shorter than and longer than the basic period. The converged values of the Wannier function and the associated energy Fourier components are analyzed, yielding improved formulae for their behavior in the important regions that are not fully asymptotic.
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