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We present a rare‐earth‐doped sapphire laser. Single‐crystalline α‐Al2O3 films doped with trivalent neodymium have been grown by pulsed laser deposition on undoped sapphire substrates. The Nd3+ doping concentrations of the films have been varied between 0.3 at.% and 2 at.%. Epitaxial growth was proven by structural and optical characterization of the films. The samples exhibit strongly polarization dependent emission transitions from the 4F3/2 manifold with a fluorescence lifetime of 108 μs and peak emission cross sections of 1.1 × 10−18 cm2 around 1100 nm. Lasing at 1096.5 nm was achieved under Ti:sapphire‐pumping in a planar waveguide configuration with a maximum cw output power of 137 mW and a slope efficiency of 7.5% with respect to the incident pump power.

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