An unsaturated Mn(II)-centered metal− organic framework was synthesized. The presence of an unsaturated Mn(II) center, together with a guestresponsive structural changing feature, plays a crucial role for strong binding with water, leading to its potential application for water/ethanol separation. In addition, the present framework is thermally stable up to 400 °C, which is beneficial for the regeneration process after adsorption.
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