We present a new formulation of Maker fringes in parallel-surface films, using self-consistent boundary conditions for reflections and allowing for any degree of refractive-index dispersion. This treatment of the second-harmonic reflections and dispersion, unlike a number of previous derivations, leads correctly to the expected form for the effective second-harmonic d coefficients. Complete expressions with physically meaningful factors are given for the generated second-harmonic power for either absorbing or birefringent films including reflections for the case of no pump depletion. A comparison with the isotropic approximation is given, and practical considerations in the use of these expressions for the fitting of experimental data are discussed.
We present new closed-form expressions for analysis of Teng-Man measurements of the electro-optic coefficients of poled polymer thin films. These expressions account for multiple reflection effects using a rigorous analysis of the multilayered structure for varying angles of incidence. The analysis based on plane waves is applicable to both transparent and absorptive films and takes into account the properties of the transparent conducting electrode layer. Methods for fitting data are presented and the error introduced by ignoring the transparent conducting layer and multiple reflections is discussed.
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