In the course of a systematic investigation of some compounds of uranium (IV), several physico‐chemical methods have been applied to the salts of the series UX4 and M2UX6 (with X = Cl, Br, I and M = Li, Na, K, Rb, Cs). ‐ The results obtained in the present work refer to UCl4; they have been obtained by electrical conductivity measurements, by differential thermal analysis and by differential enthalpic analysis.
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