A water-soluble dinuclear Cp*Ir complex bearing 4,4′,6,6′-tetrahydroxy-2,2′-bipyrimidine as a bridging ligand was found to be a highly effective catalyst for the N-alkylation of ketones with alcohols in water.

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A cyclometalated iridium(III) complex Ir(tpy)@CTF, which is designed and synthesized by the coordinative immobilization of [Ir(tpy)Cl3] on a functionalized covalent triazing framework, was proven to be a highly effective for...