Chiral quasi‐2D perovskite single crystals (SCs) were investigated for their circular polarized light (CPL) detecting capability. Quasi‐2D chiral perovskites, [(R)‐β‐MPA]2MAPb2I7 ((R)‐β‐MPA=(R)‐(+)‐β‐methylphenethylamine, MA=methylammonium), have intrinsic chirality and the capability to distinguish different polarization states of CPL photons. Corresponding quasi‐2D SCs CPL photodetector exhibit excellent detection performance. In particular, our device responsivity is almost one order of magnitude higher than the reported 2D perovskite CPL detectors to date. The crystallization dynamics of the film were modulated to facilitate its carrier transport. Parallel oriented perovskite films with a homogeneous energy landscape is crucial to maximize the carrier collection efficiency. The photodetector also exhibits superior mechanical flexibility and durability, representing a promising candidate for sensitive and robust CPL photodetectors.
Chiral quasi‐2D perovskite single crystals (SCs) were investigated for their circular polarized light (CPL) detecting capability. Quasi‐2D chiral perovskites, [(R)‐β‐MPA]2MAPb2I7 ((R)‐β‐MPA=(R)‐(+)‐β‐methylphenethylamine, MA=methylammonium), have intrinsic chirality and the capability to distinguish different polarization states of CPL photons. Corresponding quasi‐2D SCs CPL photodetector exhibit excellent detection performance. In particular, our device responsivity is almost one order of magnitude higher than the reported 2D perovskite CPL detectors to date. The crystallization dynamics of the film were modulated to facilitate its carrier transport. Parallel oriented perovskite films with a homogeneous energy landscape is crucial to maximize the carrier collection efficiency. The photodetector also exhibits superior mechanical flexibility and durability, representing a promising candidate for sensitive and robust CPL photodetectors.
High performance ultra-flexible lightweight perovskite photodetectors have promising applications on a variety of substrates, including those used on unmanned aerial vehicles. Herein, we report on a facile method to improve the performance of perovskite photodetectors on flexible ultrathin (50 μm) polyimide substrates by tuning the composition with different ratios of cations. In the presence of lead thiocyanate, the introduction of a certain amount of formamidinium could sufficiently enhance the quality of methylammonium lead triiodide perovskite film, with prolonged carrier lifetime. A perovskite photodetector with a response time of ton = 89 ms and toff = 47 ms is achieved with a very simple device architecture. In addition, our flexible photodetectors maintain good performance after rigorous folding and bending, demonstrating excellent mechanical properties, which could be very useful for a variety of applications.
In this Letter, we report an Airy-like beam of magnetostatic surface spin wave (AiBMSSW) supported on the ferromagnetic film, which is transferred from the optical field. The propagation properties of AiBMSSW were verified with micromagnetic simulation. From simulation results, the typical parabolic trajectory of the Airy-type beam was observed with an exciting source encoding 3/2 phase pattern. The simulation results coincide well with design parameters. Furthermore, simulated results showed that the trajectories of the AiBMSSW could be tuned readily with varied external magnetic fields. This work can extend the application scenario of spin waves.
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