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This study aimed at investigating the ballistic performance of Zr-based bulk metallic glass/Ti surface composites fabricated by high-energy electron-beam irradiation. The ballistic impact test was conducted on surface composite plates to evaluate the ballistic performance. Since the surface composite layers were observed to block effectively a fast traveling projectile, while many cracks were formed in the composite layers, the surface composite plates were not perforated. The surface composite layer containing ductile β dendritic phases showed the better ballistic performance than the one without containing dendrites because dendritic phases could hinder the propagation of shear bands or cracks.