The concept of “fiber art” not only expresses a kind of art but also reflects the course of this art—the evolution from a material to an art. It also reflects the characteristics of this art form—art produced by materials. This article aims to explore the application analysis of the gel method Ba2TiSi2O8 ferroelectric thin film in contemporary handicraft three-dimensional fiber art works. This article first discusses the influence of ferroelectric domains on ferroelectric thin films and concludes that domains are the basis of various physical properties and applications of ferroelectric materials. By changing the types and quantities of domains, the performance of ferroelectric materials can be controlled. Then the measurement principle of the ferromagnetic resonance line width in the ferroelectric thin film is proposed, and the Ba2TiSi2O8 ferroelectric thin film is prepared by the gel method. Then the ferromagnetism and temperature stability of the Ba2TiSi2O8 ferroelectric film are discussed, and the contemporary handicraft three-dimensional fiber art works are analyzed based on the ferroelectric film. The classical methods to detect ferromagnetic permeability tensors mainly include non-resonance method, Faraday rotation method, resonance method, resonance perturbation method, and so on. The experimental results in this paper show that the polarization strength of the flexible film at high temperature is slightly reduced. As the temperature increases, the flexible film still has a good hysteresis loop, and the saturation polarization strength does not change much. It shows that the Ba2TiSi2O8 structured flexible film has good temperature stability at about 80°C, and the contemporary handicraft three-dimensional fiber art work based on ferroelectric film not only has a good economic mechanism but also has its flexibility and beauty increased by 80%.