Additive manufacturing of bimetallic structures has become a hotspot in recent years. However, the interfaces of bimetallic structures are always the weaknesses, and cracks always occur at the interfaces. Three bimetallic samples of TA15 and Inconel 625 were manufactured by laser metal deposition, and the effect of laser power on the manufacturing quality was analyzed. Then phased array ultrasonic testing (PAUT) technique was applied for crack detection for the three samples, and metallographic analysis was employed to verify detection results. The results showed that the increase of laser power can eliminate macro-cracks at the interface of the bimetallic sample, and micro-cracks at the interface can be detected by PAUT.