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The penetration of diesel particulate filters (DPFs) in the market is growing fast. However, in the current inspection/maintenance (I/M) regulation for these vehicles, particulate emissions were capped with smoke opacity, which is incompetent to identify the excessive particle number (PN) induced by non-major DPF failures such as small cracks in substrate. This research aimed at developing a fast identification method for such malfunctioning vehicles using a low-cost condensation particle counter (CPC). To verify the effectiveness of idle PN test, 33 China-5 and China-6 heavy-duty vehicles fueled with diesel and natural gas (NG) were tested using the regulatory portable emission measurement system (PEMS) as per China-6 protocol and idle PN tests using a low-cost CPC-based system. PN emissions from China-6 vehicles with malfunctioning DPFs were at a similar level to those from China-5 vehicles (without DPF), which were significantly higher than the proper counterparts. Idle PN tests using a CPC-based system managed to identify the vehicles with DPF failures. Volumetric PN concentrations of these vehicles were much higher than those of the proper ones. This study proved that an easy, fast, and low-cost procedure could be used to screen out those high emitters with DPF failure.