The study of interacting spin systems is of fundamental importance for modern condensed matter physics. On frustrated lattices, magnetic exchange interactions cannot be simultaneously satisfied, and often give rise to competing exotic ground states 1 . The frustrated 2D ShastrySutherland lattice 2 realized by SrCu 2 (BO 3 ) 2 3 is an important test to our understanding of quantum magnetism. It was constructed to have an exactly solvable 2-spin dimer singlet ground state within a certain range of exchange parameters and frustration. While the exact dimer state and the antiferromagnetic order at both ends of the phase diagram are well known, the ground state and spin correlations in the intermediate frustration range have been widely debated 2-12 . We report here the first experimental identification of the conjectured plaquette singlet intermediate phase in SrCu 2 (BO 3 ) 2 . It is observed by inelastic neutron scattering after pressure tuning at 21.5 kbar. This gapped plaquette singlet state with strong 4-spin correlations leads to a transition to an ordered Néel state above 40 kbar, which can realize a deconfined quantum critical point.In the field of quantum magnetism, geometrically frustrated lattices generally imply major difficulties in analytical and numerical studies. For very few particular topologies however, it has been shown that the ground state, at least, can be calculated exactly as for the Majumdar-Gosh model 13 that solves the J 1 -J 2 zigzag chain when J 1 = 2J 2 . In 2D, the Shastry-Sutherland model 2 consisting of an orthogonal dimer network of spin S=1/2 was developed in order to be exactly solvable. For an inter-dimer J to intra-dimer J exchange ratio α ≡ J /J ≤ 0.5 the ground state is a product of singlets on the strong bond J. Numerical calculations have further shown that this remains valid up to α ≤∼ 0.7 and for small values of 3D couplings J between dimer layers. At the other end, for ∼ 0.9 ≤ α ≤ ∞ the system approaches the well known 2D square lattice, which is antiferromagnetically (AFM) ordered, albeit with significant quantum fluctuations that are believed to include resonating singlet correlations resulting in fractional excitations 14 . The phase diagram of the Shastry-Sutherland model, both with and without applied magnetic field, has been intensively studied by numerous theoretical and numerical approaches 3 . In the presence of magnetic field, magnetization plateaus at fractional values of the saturation magnetization corresponding to Mott insulator phases of dimer states, as well as possible superfluid and supersolid phases have been extensively studied 6,15,16 . At zero field, the main unsolved issue is the existence and nature arXiv:1603.02039v1 [cond-mat.str-el]
Magnetic susceptibility measurements have shown that the compounds Mn(1-x)Fe(x)Ge are magnetically ordered through the whole range of concentrations x = [0.0,1.0]. Small-angle neutron scattering reveals the helical nature of the spin structure with a wave vector, which changes from its maximum (|k| = 2.3 nm(-1)) for pure MnGe, through its minimum (|k| → 0) at x(c) ≈ 0.75, to the value of |k| = 0.09 nm(-1) for pure FeGe. The macroscopic magnetic measurements confirm the ferromagnetic nature of the compound with x = x(c). The observed transformation of the helix structure to the ferromagnet at x = x(c) is explained by different signs of chirality for the compounds with x > x(c) and x
We carried out hydrostatic pressure demagnetization experiments up to 1.24 GPa on samples of terrestrial and extraterrestrial rocks and minerals of different lithologies as well as on synthetic samples. The magnetic remanence of samples was measured directly under pressure using a non-magnetic high pressure cell of piston-cylinder type that was inserted into a high sensitivity SQUID magnetometer. In order to bring light on the pressure demagnetization effect, we investigated 50 samples with different magnetic mineralogies, remanent coercivities (B cr) and hysteresis parameters. The samples consisted of pyrrhotite-, magnetite-and titanomagnetite-bearing Martian meteorites, taenite-, tetrataenite and kamacite-bearing ordinary chondrites and pyrrhotite-bearing Rumuruti chondrite; magnetite-and titanomagnetite-bearing basalts, andesites, ignimbrites, obsidians and granites; a variety of pyrrhotite-and hematite-bearing rocks and minerals (jasper, schist, rhyolite, radiolarite); samples of goethite and greigite as well as synthetic samples of dispersed powders of magnetite, hematite, pyrrhotite and native iron set into epoxy resin. Under hydrostatic pressure of 1.24 GPa, applied in a low magnetic field (<5µT), the samples lost up to 84% of their initial saturation isothermal remanent magnetization (SIRM) without any changes in their intrinsic magnetic properties. We found that the efficiency of the pressure demagnetization is not exclusively controlled by the magnetic hardness of the samples (B cr), but that it is strongly dependent on their magnetic mineralogy. For a given magnetic mineralogy the resistance to hydrostatic pressure is roughly proportional to ln(B cr). It was shown that there is no simple equivalence between pressure demagnetization and alternating field demagnetization effects. The
We determined the hydrostatic limits at room temperature for a number of Fluorinert liquids: FC70, FC75, FC77, FC84, FC87 and their mixtures. Pressure exceeding this limit produces pressure gradients in the sample, which are retained at low temperature. The maximum hydrostatic limit (2.3 GPa) was found for a (1:1) mixture of FC84/87. 1 3M TM Fluorinert TM liquids for Electronics Manufacturing (selection guide).
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