A bottom-up framework to investigate environmental and techno-economic aspects of lithium-ion batteries: A case study of conventional vs. pre-lithiated lithium-ion battery cells

Orangi, Sina; Manjong, Nelson Bunyui; Clos, Daniel Perez; Burheim, Odne Stokke; Strømman, Anders Hammer

doi:10.1016/j.jclepro.2024.143934

Journal of Cleaner Production

2024

DOI: 10.1016/j.jclepro.2024.143934

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A bottom-up framework to investigate environmental and techno-economic aspects of lithium-ion batteries: A case study of conventional vs. pre-lithiated lithium-ion battery cells

Sina Orangi,

Nelson Bunyui Manjong,

Daniel Perez Clos

et al.

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Quantifying Lithium-Ion Battery Rate Capacity, Electrode Structuring, and Transport Phenomena Using E-I Measurements

Dunne,

Solberg,

Amiri

et al. 2024

Batteries

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The specific energy of lithium-ion batteries (LIBs) can be enhanced through various approaches, one of which is increasing the proportion of active materials by thickening the electrodes. However, this typically leads to the battery having lower performance at a high cycling rate, a phenomenon commonly known as rate capacity retention. One solution to this is perforating the electrode, by creating channels or corrugations in the active electrode material, either as holes or as channels. This is known to reduce the rate capacity retention effect, but in order to engineer this better, a simplified transport process analysis needs to be established. In this paper, we propose a classic electrochemical analysis based on voltage–charge cycling measurements in order to obtain a classical mass transport coefficient, hm, that is further used as a main indicator for electrode design quality assessment. We also demonstrate theoretically and experimentally how the mass transfer coefficient, hm, can be determined and how it changes as the electrode layer thickness increases, with and without electrode corrugations.

show abstract

Quantifying Lithium-Ion Battery Rate Capacity, Electrode Structuring, and Transport Phenomena Using E-I Measurements

Dunne,

Solberg,

Amiri

et al. 2024

Batteries

View full text Add to dashboard Cite

show abstract

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A bottom-up framework to investigate environmental and techno-economic aspects of lithium-ion batteries: A case study of conventional vs. pre-lithiated lithium-ion battery cells

Cited by 1 publication

References 66 publications

Quantifying Lithium-Ion Battery Rate Capacity, Electrode Structuring, and Transport Phenomena Using E-I Measurements

Quantifying Lithium-Ion Battery Rate Capacity, Electrode Structuring, and Transport Phenomena Using E-I Measurements

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