1999
DOI: 10.1016/s0009-2509(99)00007-x
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A concept to simulate an industrial size tube reactor with fast complex kinetics and absorption of two gases on the basis of CFD modeling

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Cited by 10 publications
(3 citation statements)
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“…We performed pH measurements for the individual species dissolved in the aqueous phase and the organic phase, in Table 1 The potential reactions considered in this work are summarized along-with the required criteria Potential reactions Criteria Remarks 1 2 3 4 Phase transfer catalysis reaction N N Y Y Does not satisfy required (Dehmlow & Dehmlow, 1993;criteria Weber and Gokel, 1977) Selective non-catalytic reduction reaction Y Y Y N (Park et al, 1996;Sun et al, 2001; Complex free radical reaction Miller and Klippenstein (2000)) Simultaneous absorption of two gases Y Y Y N L o w sensitivity of gaseous (Warnecke et al, 1999; reactants for spectroscopic Ramachandran & Sharma, 1971) measurement Weak acid-weak base equilibrium Y Y Y Y Satisfies all the required criteria reaction Weak acid-weak base equilibrium reaction is found to be the most appropriate reaction. In the above table, Y indicates that respective criterion is satisfied while N indicates that respective criterion is not satisfied.…”
Section: Selected Reactionmentioning
confidence: 99%
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“…We performed pH measurements for the individual species dissolved in the aqueous phase and the organic phase, in Table 1 The potential reactions considered in this work are summarized along-with the required criteria Potential reactions Criteria Remarks 1 2 3 4 Phase transfer catalysis reaction N N Y Y Does not satisfy required (Dehmlow & Dehmlow, 1993;criteria Weber and Gokel, 1977) Selective non-catalytic reduction reaction Y Y Y N (Park et al, 1996;Sun et al, 2001; Complex free radical reaction Miller and Klippenstein (2000)) Simultaneous absorption of two gases Y Y Y N L o w sensitivity of gaseous (Warnecke et al, 1999; reactants for spectroscopic Ramachandran & Sharma, 1971) measurement Weak acid-weak base equilibrium Y Y Y Y Satisfies all the required criteria reaction Weak acid-weak base equilibrium reaction is found to be the most appropriate reaction. In the above table, Y indicates that respective criterion is satisfied while N indicates that respective criterion is not satisfied.…”
Section: Selected Reactionmentioning
confidence: 99%
“…Instead, the two reactants diffuse into a dispersed phase that is introduced, where the reaction takes place, e.g. manufacturing of propylene oxide (Warnecke et al, 1999) and proton exchange reactions. In the present work, we are interested in the latter case.…”
Section: Introductionmentioning
confidence: 99%
“…Important recent developments in gas absorption with reaction deal with the more advanced cases of multiple gases in contrast to earlier emphasis on the single gas case . A number of key works have covered the simultaneous absorption and reaction of two gases. More recently, the case of three gases has been addressed, , although the frequently studied absorption of NO x involves four gaseous components . There is however no general theory yet available for multicomponent gas absorption with reaction(s).…”
Section: Introductionmentioning
confidence: 99%