A fully-printed electrochemical platform for assisted colorimetric detection of phosphate in saliva: Greenness and whiteness quantification by the AGREE and RGB tools

Mazzaracchio, Vincenzo; Sassolini, Alessandro; Mitra, Kalyan Yoti; Mitra, Dana; Stojanović, Goran M.; Willert, Andreas; Sowade, Enrico; Baumann, Reinhard R.; Zichner, Ralf; Moscone, Danila; Arduini, Fabiana

doi:10.1016/j.greeac.2022.100006

Cited by 14 publications

(4 citation statements)

References 39 publications

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“…The key decision criteria were selected in accordance with the 12 principles of green analytical chemistry. These criteria include the use of direct analytical techniques, the use of small sample size, in situ measurements, step numbers, automation and miniaturization, derivatization, waste generation, multianalyte, energy minimization, renewable reagents, toxic reagents, and safety for operator (Mazzaracchio et al 2022 ). GAC principles were translated into 0–1 AGREE calculator scores (default weighting) using the input data for the 12 decision criteria.…”

Section: Methodsmentioning

confidence: 99%

Multi-criteria decision analysis: technique for order of preference by similarity to ideal solution for selecting greener analytical method in the determination of mifepristone in environmental water samples

Makwakwa,

Moema,

Msagati

2024

Environ Sci Pollut Res

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This work proposes the use of multi-criteria decision analysis (MCDA) to select a more environmentally friendly analytical procedure. TOPSIS, which stands for Technique for Order of Preference by Similarity to Ideal Solution, is an example of a MCDA method that may be used to rank or select best alternative based on various criteria. Thirteen analytical procedures were used in this study as TOPSIS input choices for mifepristone determination in water samples. The input data, which consisted of these choices, was described using assessment criteria based on 12 principles of green analytical chemistry (GAC). Based on the objective mean weighting (MW), the weights for each criterion were assigned equally. The most preferred analytical method according to the ranking was solid phase extraction with micellar electrokinetic chromatography (SPE-MEKC), while solid phase extraction combined with ultra-high performance liquid chromatography tandem mass spectrometry (SPE-UHPLC-MS/MS) was ranked last. TOPSIS ranking results were also compared to the green metrics NEMI, Eco-Scale, GAPI, AGREE, and AGREEprep that were used to assess the greenness of thirteen analytical methods for mifepristone determination. The results demonstrated that only the AGREE metric tool correlated with TOPSIS; however, there was no correlation with other metric tools. The analysis results suggest that TOPSIS is a very useful tool for ranking or selecting the analytical procedure in terms of its greenness and that it can be easily integrated with other green metrics tools for method greenness assessment.

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Section: Methodsmentioning

confidence: 99%

Multi-criteria decision analysis: technique for order of preference by similarity to ideal solution for selecting greener analytical method in the determination of mifepristone in environmental water samples

Makwakwa,

Moema,

Msagati

2024

Environ Sci Pollut Res

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“…In 2021, I proposed the idea of "white analytical chemistry (WAC)", 27 which has already met with a positive reception in the GAC environment. [28][29][30][31][32] This concept joins greenness, sustainability and performance-related criteria:…”

Section: Green Sustainable Or… White?mentioning

confidence: 99%

What does it mean that “something is green”? The fundamentals of a Unified Greenness Theory

Nowak

2023

Green Chem.

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“…The proposed method is rated green by the EcoScale Green Assessment Tool with a score of 86 (excellent green method) and a score of 0.46 obtained using AGREE tool. To support the colorimetric detection of phosphate in saliva, Mazzaracchio et al 184 evaluated the greenness and whiteness of a fully printed electrochemical platform using the AGREE and RGB tools, and the final score of the AGREE assessment is 0.73 out of a total score of 1. A greenness assessment of the sample preparation method for the green electromembrane extraction procedure based on biodegradable chitosan films to identify polyphenolic compounds in food samples was carried out by Roman-Hidalgo et al , 185 who evaluated the environmental friendliness of the sample preparation method for the green electromembrane extraction procedure based on biodegradable chitosan films for the identification of polyphenolic compounds in food samples.…”

Section: Green Metrics and Morementioning

confidence: 99%

Greener chemistry in analytical sciences: from green solvents to applications in complex matrices. Current challenges and future perspectives: a critical review

Ražić¹,

Arsenijević²,

Mračević³

et al. 2023

Analyst

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A fully-printed electrochemical platform for assisted colorimetric detection of phosphate in saliva: Greenness and whiteness quantification by the AGREE and RGB tools

Cited by 14 publications

References 39 publications

Multi-criteria decision analysis: technique for order of preference by similarity to ideal solution for selecting greener analytical method in the determination of mifepristone in environmental water samples

Multi-criteria decision analysis: technique for order of preference by similarity to ideal solution for selecting greener analytical method in the determination of mifepristone in environmental water samples

What does it mean that “something is green”? The fundamentals of a Unified Greenness Theory

Greener chemistry in analytical sciences: from green solvents to applications in complex matrices. Current challenges and future perspectives: a critical review

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