2017
DOI: 10.1021/acs.nanolett.7b04050
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A Gallium-Based Magnetocaloric Liquid Metal Ferrofluid

Abstract: We demonstrate a magnetocaloric ferrofluid based on a gadolinium saturated liquid metal matrix, using a gallium-based liquid metal alloy as the solvent and suspension medium. The material is liquid at room temperature, while exhibiting spontaneous magnetization and a large magnetocaloric effect. The magnetic properties were attributed to the formation of gadolinium nanoparticles suspended within the liquid gallium alloy, which acts as a reaction solvent during the nanoparticle synthesis. High nanoparticle weig… Show more

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Cited by 122 publications
(88 citation statements)
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“…Many LM‐X mixtures (X being the solid particle filler) are actively investigated to expand the functional capabilities of LMs not only in thermal management of electronics but also in other applications including wearables and soft robotics. Recent reports mention successful fabrication of LM‐X mixtures that include microparticles of Cu, Fe, Ni, Ag, Mg, Gd, BN, Cu–Fe, steel, diamond, graphene, and carbon nanotubes . Controlling the fraction of solid additives can facilitate a desirable transition from a liquid‐like to paste‐like rheology for these mixtures that is easily spread on a surface.…”
mentioning
confidence: 99%
“…Many LM‐X mixtures (X being the solid particle filler) are actively investigated to expand the functional capabilities of LMs not only in thermal management of electronics but also in other applications including wearables and soft robotics. Recent reports mention successful fabrication of LM‐X mixtures that include microparticles of Cu, Fe, Ni, Ag, Mg, Gd, BN, Cu–Fe, steel, diamond, graphene, and carbon nanotubes . Controlling the fraction of solid additives can facilitate a desirable transition from a liquid‐like to paste‐like rheology for these mixtures that is easily spread on a surface.…”
mentioning
confidence: 99%
“…The addition of Fe 3 O 4 nanoparticles was put. through vigorous stirring, which is a common strategy of incorporating magnetic nanoparticles [114][115][116]. The magnetic torque acting on the micromotor can be described by…”
Section: Magnetic Propulsionmentioning
confidence: 99%
“…For soft polymer devices like those presented here, this can readily lead to thermal failure, due to the inefficient thermal transport of elastomers, and becomes a limiting factor. One method for reducing heating is to enhance the electrical conductivity of the liquid metal by suspending conductive (silver or gold) nanoparticles in it using one of several previous described techniques . The resulting solutions are invariably high in viscosity, making them difficult to introduce into solid substrates.…”
Section: Development Of a Soft 3d Electromagnetic Inductormentioning
confidence: 99%