2024
DOI: 10.1002/advs.202310035
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A High‐Density Hydrogen Bond Locking Strategy for Constructing Anisotropic High‐Strength Hydrogel‐Based Meniscus Substitute

Qian Zhang,
Xuxuan Yang,
Kuan Wang
et al.

Abstract: Mimicking anisotropic features is crucial for developing artificial load‐bearing soft tissues such as menisci). Here, a high‐density hydrogen bond locking (HDHBL) strategy, involving preloading a poly(N‐acryloylsemicarbazide) (PNASC) hydrogel with an aqueous solution containing a hydrogen bond breaking agent, followed by water exchange, to fabricate anisotropic high‐strength hydrogels are proposed. During this process, multiple high‐density hydrogen bonds of the PNASC network are re‐established, firmly freezin… Show more

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