2019
DOI: 10.1073/pnas.1911021116
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A multifunctional shape-morphing elastomer with liquid metal inclusions

Abstract: Natural soft tissue achieves a rich variety of functionality through a hierarchy of molecular, microscale, and mesoscale structures and ordering. Inspired by such architectures, we introduce a soft, multifunctional composite capable of a unique combination of sensing, mechanically robust electronic connectivity, and active shape morphing. The material is composed of a compliant and deformable liquid crystal elastomer (LCE) matrix that can achieve macroscopic shape change through a liquid crystal phase transiti… Show more

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Cited by 250 publications
(220 citation statements)
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“…LMs are also utilized for electrical applications, due to their huge (relative to other options) electrical conductivity and dielectric properties (e.g., refs. [ 12,115,152–155 ] , Figure 5D). In general, most as‐fabricated, discrete liquid in continuous solid/liquid metal composites are insulating, both due to the insulating elastomer phase, and due to insulating oxide layers around the LM droplets.…”
Section: Properties Of Slcsmentioning
confidence: 99%
See 1 more Smart Citation
“…LMs are also utilized for electrical applications, due to their huge (relative to other options) electrical conductivity and dielectric properties (e.g., refs. [ 12,115,152–155 ] , Figure 5D). In general, most as‐fabricated, discrete liquid in continuous solid/liquid metal composites are insulating, both due to the insulating elastomer phase, and due to insulating oxide layers around the LM droplets.…”
Section: Properties Of Slcsmentioning
confidence: 99%
“…Upon the application of large voltages, the Maxwell stress pulls the outer surfaces together which also produces deformations outside of the active electrode area which can be leveraged to do rapid work. Further approaches include actuation via electrohydrodynamic pumping of liquid within elastomeric channels, [ 215 ] embedding of LM droplets into liquid crystal elastomers (LCEs) to enable electrically activated shape‐shifting structures (Figure 9G), [ 154 ] and encapsulating electrically controlled, shape‐memory‐alloy (SMA) wires in LM/elastomer composites. In this last case, the composite material serves to give low mechanical resistance to actuation, which enhances the actuation frequency and deflection, while dissipating heat generated by the SMA wires.…”
Section: Applicationsmentioning
confidence: 99%
“…[73] Recently, Majidi and coworkers reported an electrothermal LCN composite with dispersed liquid metal (LM) microdroplets. [74] Unlike the previous LCN composites with rigid components, the liquid state of LM allows the LCN to maintain its mechanical compliance even with up to 50 vol% of LM. The high content of LM in the LCN improves the thermal and electrical conductivity of the material, which ensures large reversible deformation at relatively low voltage.…”
Section: Electro-responsive Lcnsmentioning
confidence: 99%
“…Except for heat, topographical features of LCE sheets can also be controlled with either light [ 66 ] or electrical stimulation. [ 50,67,68 ]…”
Section: Surface Morphingmentioning
confidence: 99%