Abstract:The intriguing functionalities of emerging quasi-two-dimensional (2D) metal halide perovskites (MHPs) have led to further exploration of this material class for sustainable and scalable optoelectronic applications. However, the chemical complexities in precursors – primarily determined by the 2D:3D compositional ratio – results in the uncontrolled phase heterogeneities in these materials, which compromises the optoelectronic performances. Yet, this phenomenon remains poorly understood due to the massive quasi-… Show more
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