2023
DOI: 10.1002/chem.202301774
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Amorphous TiO2 shells: an Essential Elastic Buffer Layer for High‐Performance Self‐Healing Eutectic GaSn Nano‐Droplet Room‐Temperature Liquid Metal Battery

Abstract: Gallium‐based alloy liquid metal batteries currently face limitations such as volume expansion, unstable solid electrolyte interface (SEI) film and substantial capacity decay. In this study, amorphous titanium dioxide is used to coat eutectic GaSn nanodroplets (eGaSn NDs) to construct the core‐shell structure of eGaSn@TiO2 nanodroplets (eGaSn@TiO2 NDs). The amorphous TiO2 shell (~6.5 nm) formed a stable SEI film, alleviated the volume expansion, and provided electron/ion transport channels to achieve excellent… Show more

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