An experimental and kinetic modeling study of the auto-ignition delay times of trimethyl phosphate-in-air mixtures

Bruce, Frederick Nii Ofei; He, Ruining; Xuan, Ren; Xin, Bai; Ma, Yue; Li, Yang

doi:10.1016/j.jaecs.2023.100237

Applications in Energy and Combustion Science

2024

DOI: 10.1016/j.jaecs.2023.100237

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An experimental and kinetic modeling study of the auto-ignition delay times of trimethyl phosphate-in-air mixtures

Frederick Nii Ofei Bruce,

Ruining He,

Ren Xuan

et al.

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Low-Gassing, Non-Flammable Liquid Electrolyte for Anode-Free Batteries

Rajendran,

Abraham,

Xie

et al. 2024

J. Electrochem. Soc.

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Lithium metal and anode-free batteries are generating significant interest due to their remarkably high energy density in a compact size, paving the way for extended range in electric vehicles. However, the high-voltage cathode and reactive lithium metal anode tend to catalyze the decomposition of conventional carbonate and ether-based electrolytes, leading to significant gassing, swelling, and rapid capacity fade. Additionally, these electrolytes contain one or more highly flammable components, reducing the overall safety by acting like a fuel during a thermal event. Here, we highlight the use of a non-flammable localized high-concentration electrolyte based on Triethyl Phosphate in a Copper (Cu) || LiNi0.8Mn0.1Co0.1O2 (NMC811) stacked pouch cell. This proposed electrolyte combination significantly reduces gassing, maintains non-flammability, and does not compromise on cycle life.

show abstract

Low-Gassing, Non-Flammable Liquid Electrolyte for Anode-Free Batteries

Rajendran,

Abraham,

Xie

et al. 2024

J. Electrochem. Soc.

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show abstract

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An experimental and kinetic modeling study of the auto-ignition delay times of trimethyl phosphate-in-air mixtures

Cited by 1 publication

References 80 publications

Low-Gassing, Non-Flammable Liquid Electrolyte for Anode-Free Batteries

Low-Gassing, Non-Flammable Liquid Electrolyte for Anode-Free Batteries

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