2024
DOI: 10.1002/smll.202405143
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Asymmetrical Functionalization of Polarizable Interface Restructuring Molecules for Rapid and Longer Operative Lithium Metal Batteries

Chae Yeong Son,
Daehyun Kim,
Seo‐Young Jun
et al.

Abstract: Lithium metal batteries (LMBs) have been recognized as high‐energy storage alternatives; however, problematic surface reactions due to dendritic Li growth are major obstacles to their widespread utilization. Herein, a 3‐mercapto‐1‐propanesulfonic acid sodium salt (MPS) with asymmetrically functionalized thiol and sulfonate groups as polarizable interface‐restructuring molecules is proposed to achieve rapid and longer‐operating LMBs. Under a harsh condition of 5 mA cm−2, Li–Li symmetric cells employing MPS can … Show more

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