Airport areas generate significant air pollution from both air and surface traffic. Policy makers often address this by considering single contributions, either from rubber-tired vehicles or aircraft, leading to an underestimation of the non-considered-mode’s impact. Similarly, literature on airport pollution often focuses on specific case studies, evaluating either surface or air traffic. Understanding the overlap of these contributions requires calculation of emissions from both traffic modes. This raises two research questions: which is the major contributor, and what mitigation measures can be applied? This paper addresses these questions through two Italian case studies. In the first, we estimated emissions from passenger cars, buses, and aircraft in a medium-sized airport representative of similar facilities across Italy and Europe, calculating emissions using COPERT for surface modes and ICAO methodologies for each LTO cycle. Results showed that aircraft emissions were significantly higher than those from surface vehicles. To address this, the second case study examined four mitigation measures at take-off and landing at another Italian airport, recalculating emissions via the same methodologies. The paper details the methodology process, presents results, and discusses the management of air-operations’ effects at urban airports within local mobility policies and practice, all within the research goal of advancing knowledge farther afield.