Binaphthyl-containing electroactive polymer networks by ring-opening metathesis polymerization

Yang, Ki Seok; Jeong, Dong−Cheol; Choi, Eun Jung; Ahn, Tae-Kyu; Song, Changsik

doi:10.1007/s13233-013-1172-9

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“…The polymerizable monomer BT-NHC-AuCl was designed and synthesized (Scheme ). The introduction of bithiophene (BT) units renders the monomer BT-NHC-AuCl polymerizable under oxidative conditions. , Cowley and co-workers reported an electropolymerizable NHC-Au complex, where two BTs were directly attached to the backside carbons of the heterocycle . Our design was to affix BTs at the periphery of N-aryl groups of the NHC owing to its synthetic modularity.…”

Section: Resultsmentioning

confidence: 99%

N-Heterocyclic Carbene-Based Conducting Polymer–Gold Nanoparticle Hybrids and Their Catalytic Application

Song¹,

Satheeshkumar²,

Park³

et al. 2014

Macromolecules

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Hybrid nanocomposites of N-heterocyclic carbene (NHC)-functionalized conducting polymers (CPs) with gold nanoparticles (AuNPs) were prepared by concurrent disproportionation and oxidative coupling. The formation of hybrid nanocomposites, NHC-CP/AuNPs, in the simultaneous process was confirmed by transmission electron microscopy, powder X-ray diffraction, cyclic voltammetry, and 13C solid-state NMR analyses. More importantly, the NHC group played a pivotal role in the dispersion of AuNPs. Further, NHC-CP/AuNPs exhibited good catalytic activity for the reduction of 4-nitrophenol.

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Section: Resultsmentioning

confidence: 99%