Biomass derived sulfonated carbon catalysts: efficient catalysts for green chemistry

Zhu, Shangkun; Ke, Jian; Li, Xiang; Zheng, Zixuan; Guo, Ruixin; Chen, Jianqiu

doi:10.1039/d4gc00113c

Green Chem.

2024

DOI: 10.1039/d4gc00113c

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Biomass derived sulfonated carbon catalysts: efficient catalysts for green chemistry

Shangkun Zhu,

Jian Ke,

Xiang Li

et al.

Abstract: BDSCCs, known as efficient solid acid catalysts with easy preparation and a green source, are anticipated to play a role in advancing circular and economic development in various sectors.

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Cited by 6 publications

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Recent Advances in the Synthesis of 2‐Furoic Acid and 2,5‐Furandicarboxylic Acid from Furfural

Zhang,

Cui,

Xia

2024

ChemSusChem

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2,5‐furandicarboxylic acid (FDCA) is an important organic platform compound that has been widely used in the fields of medicine, pesticides, dyes, plastics and resins due to its unique structure and properties. In recent years, with the emphasis on sustainable development and green chemistry, the synthesis of FDCA from biomass has attracted extensive attention. The catalytic conversion of furfural (FF) to FDCA has the advantages of easy availability of the raw material, environmental friendliness, economic feasibility and so on, which is an important direction for FDCA synthesis in the future. This paper mainly reviews the prepare pathways of furoic acid (FA) and FDCA using FF as a starting material, including the selective conversion of FF and FA to target products under different types of catalysts. First, the research progress in the synthesis of FA from FF was summarized, and then the advances in the catalytic conversion of FA to FDCA was reviewed. In addition, the development of efficient and green catalysts and the optimization of existing synthesis protocols are emphasized as key factors to improve the yield and purity of FDCA while reducing production costs. Finally, the opportunities and challenges were discussed.

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Recent Advances in the Synthesis of 2‐Furoic Acid and 2,5‐Furandicarboxylic Acid from Furfural

Zhang,

Cui,

Xia

2024

ChemSusChem

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Ni/PiNe Heterogeneous Catalyst from Biomass Waste: Low‐Loading, Ligand‐Free Suzuki‐Miyaura Cross‐Coupling

Valentini,

Chen,

Brufani

et al. 2024

ChemSusChem

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An efficient Ni‐based heterogeneous catalyst from pine needles urban waste valorization was designed and developed with a resource recycling strategy. The Ni/PiNe catalyst was fully characterized and tested in the Suzuki‐Miyaura coupling under microwave irradiation. Although Ni is a promising candidate for replacing Pd‐based catalytic systems, it generally requires a high catalyst amount and the exploitation of ligands and additives to enhance the reaction rate. On the contrary, with our new Ni/PiNe, 30 different products were efficiently synthesized with an isolated yield of up to 93%, using a very low catalyst amount and in the absence of ligands. Furthermore, the Ni/PiNe catalyst also showed good durability for consecutive cycles and an impressive TON value (1140). In addition to the catalytic efficiency in short reaction time and to the stability and durability under MW irradiation, the Ni/PiNe allowed for further optimization, achieving a low E‐factor value (14.0), thus highlighting the potential in further reducing the waste and costs associated to the process.

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3D-Printing Functional Ceramic for One-Step Fabrication of Pd/C Catalytic Reactor

Wu,

Xu,

Zhang

et al. 2024

Additive Manufacturing Frontiers

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Biomass derived sulfonated carbon catalysts: efficient catalysts for green chemistry

Abstract: BDSCCs, known as efficient solid acid catalysts with easy preparation and a green source, are anticipated to play a role in advancing circular and economic development in various sectors.

Cited by 6 publications

References 132 publications

Recent Advances in the Synthesis of 2‐Furoic Acid and 2,5‐Furandicarboxylic Acid from Furfural

Recent Advances in the Synthesis of 2‐Furoic Acid and 2,5‐Furandicarboxylic Acid from Furfural

Ni/PiNe Heterogeneous Catalyst from Biomass Waste: Low‐Loading, Ligand‐Free Suzuki‐Miyaura Cross‐Coupling

3D-Printing Functional Ceramic for One-Step Fabrication of Pd/C Catalytic Reactor

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