Abstract:Designing highly efficient and stable electrode-electrolyte interface for hydrogen peroxide (H 2 O 2 ) electrosynthesis remains challenging. Inhibiting the competitive side reaction, 4 e À oxygen reduction to H 2 O, is essential for highly selective H 2 O 2 electrosynthesis. Instead of hindering excessive hydrogenation of H 2 O 2 via catalyst modification, we discover that adding a hydrogen-bond acceptor, dimethyl sulfoxide (DMSO), to the KOH electrolyte enables simultaneous improvement of the selectivity and … Show more
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