2024
DOI: 10.1021/jacs.4c02324
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Cation Distribution and Anion Transport in the La3Ga5–xGe1+xO14+0.5x Langasite Structure

Lucia Corti,
Ivan Hung,
Amrit Venkatesh
et al.

Abstract: Exploration of compositional disorder using conventional diffraction-based techniques is challenging for systems containing isoelectronic ions possessing similar coherent neutron scattering lengths. Here, we show that a multinuclear solid-state Nuclear Magnetic Resonance (NMR) approach provides compelling insight into the Ga 3+ /Ge 4+ cation distribution and oxygen anion transport in a family of solid electrolytes with langasite structure and La 3 Ga 5−x Ge 1+x O 14+0.5x composition. Ultrahigh field 71 Ga Magi… Show more

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