“…The general deterioration of river water quality has become one of the most serious environmental threats to human health and ecosystem services nationwide (Zhou et al 2017, Ma et al 2020b, Huang et al 2021. This situation is more serious in North China, where deficient water resources increasingly impede the control of water pollution and the improvement of water quality (Wang et al 2019, Ma et al 2020a, Huang et al 2021, Sun et al 2021, leading to water-pollution-induced severe water scarcity, for which this area has become a hot spot on a worldwide scale (Liu and Raven 2010, Guan et al 2014, Zhao et al 2015, Sun et al 2021. The increased demand for water to support irrigation, industry, and domestic life has nearly dried up all the natural runoff of the Hai River Basin (HRB) in North China, an area that accounts for 10% and 12% of the national population and the GDP, respectively , Xia et al 2012, and failed to eliminate the accumulated water pollutants (Guan et al 2014).…”